Surface & interface phonons
Vibrational states at free surfaces, buried interfaces, and atomically thin films, including localized and hybridized modes.
We study how atomic vibrations at surfaces and interfaces impact the properties of thin films and nanostructures. Our work combines epitaxial growth, in situ synchrotron radiation scattering and spectroscopy, and first-principles calculations to reveal how size, strain, bonding, and reduced dimensionality reshape the phonon spectra of functional nanomaterials.
The central question is how reduced dimensionality, surfaces, interfaces, and bonding modify atomic motion — and how these changes can be used to control materials properties.
Vibrational states at free surfaces, buried interfaces, and atomically thin films, including localized and hybridized modes.
Dimensional crossover from bulk crystals to ultrathin films, nanoislands, and nanowires.
Interactions between lattice vibrations, charge, spin, magnetism, entropy, and functional response.
Designing vibrational spectra for thermal management, energy materials, nanoelectronics, and quantum technologies.
They possess modified force constants, localized vibrational states, and energy-transfer pathways that can govern the macroscopic behavior of nanoscale systems.
How do bonding, strain, roughness, intermixing, and symmetry breaking create non-bulk phonon spectra?
Which phonons carry heat along and across surfaces and interfaces, and how can their propagation be controlled?
How do phonons govern electronic, magnetic, elastic, and thermodynamic properties of nanoscale materials?
How can element-specific phonon spectroscopy and modelling guide phonon-engineered nanomaterials?
Our approach combines atomically controlled samples preparation with element-specific phonon spectroscopy and quantitative lattice dynamics calculations.
Original publication:
Phonons in Epitaxial DySi2: From the Bulk to Self-Organized Nanoislands and Nanowires Phys. Rev. Lett. 135, 256202 (2025) Full publication list →
We train next generation scientists for industrial research and academia.
Co-lecturer for the following courses in the Master's program of the Faculty of Physics, KIT.
ESRF User Meeting 2026, Tutorial on Lattice dynamics and nuclear inelastic scattering.
First-principles calculations are used to study lattice dynamics, Raman spectra, phonon lifetimes, frequency shifts, and phonon-mediated heat transport in semiconductor β-FeSi₂.
Full publication list →Please contact me directly for more details.
Contact →The group is financially supported by the Initiative and Networking Funds of the President of the Helmholtz Association and the Karlsruhe Institute of Technology (contract VH-NG-625) and by the Federal Ministry of Research, Technology and Space BMFTR via the Verbundprojekt NUKFER (contract 05K16VK4) and the Verbundprojekt LANRS (contract 05K22VK2).
Please contact me directly for reprints or other queries.